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- W4387244847 abstract "Abstract We numerically and analytically investigate the behavior of a non-equilibrium phase transition in the second Schlögl 
autocatalytic reaction scheme. 
Our model incorporates both an interaction-induced phase separation and a bifurcation in the reaction kinetics, with 
these critical lines coalescing at a bicritical point in the macroscopic limit. 
We construct a stochastic master equation for the reaction processes to account for the presence of mutual particle 
interactions in a thermodynamically consistent manner by imposing a generalized detailed balance condition, which 
leads to exponential corrections for the transition rates. 
In a non-spatially extended (zero-dimensional) setting, we treat the interactions in a mean-field approximation, and
introduce a minimal model that encodes the physical behavior of the bicritical point and permits the exact evaluation of 
the anomalous scaling for the particle number fluctuations in the thermodynamic limit. 
We obtain that the system size scaling exponent for the particle number variance changes from β 0 = 3/2 at the 
standard non-interacting bifurcation to β = 12/7 at the interacting bicritical point. 
The methodology developed here provides a generic route for the quantitative analysis of fluctuation effects in chemical
reactions occurring in multi-component interacting systems." @default.
- W4387244847 created "2023-10-03" @default.
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- W4387244847 date "2023-10-02" @default.
- W4387244847 modified "2023-10-10" @default.
- W4387244847 title "Stochastic analysis of chemical reactions in multi-component interacting systems at criticality" @default.
- W4387244847 doi "https://doi.org/10.1209/0295-5075/acff15" @default.
- W4387244847 hasPublicationYear "2023" @default.
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