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• W4387306729 abstract "Abstract The performance of electric double-layer capacitors and lithium-ion batteries deteriorates with increasing humidity. The desirable effect of bound water on the energy-storage properties of physically dry cellulose nanofiber (Na-ACF) supercapacitors with sodium (Na) carboxylate radicals was investigated using infrared and near-infrared spectroscopy, and nuclear magnetic resonance spectroscopy, alternating current impedance analyses, and first-principles calculations. The storage capacity decreased gradually upon heating to 423 K and reached zero upon exceeding 483 K, accompanied by increasing electrical resistance, forming a distorted semicircle in Nyquist diagram and drawing the phase angle to zero in Bode diagram. This is attributed to the water in the hydration gel bound to the Na + -ions that cross-link the cellulose chains, evaporating as the temperature increases, and finally becoming Na 2 O. The increased band-gap energy from the increase in bound water prevents leakage from the supercapacitor. In contrast to ordinary batteries, bound water is necessary for developing Na-ACF supercapacitors." @default.
• W4387306729 created "2023-10-04" @default.
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• W4387306729 date "2023-10-03" @default.
• W4387306729 modified "2023-10-16" @default.
• W4387306729 title "High-energy storage capacity of cellulose nanofiber supercapacitors using bound water" @default.
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• W4387306729 doi "https://doi.org/10.1038/s41598-023-43222-7" @default.
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