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• W4387325892 abstract "Construction of gold-based metal-organic frameworks (Au-MOFs) would bring the merits of gold chemistry into MOFs. However, it still remains challenging because gold cations are easily reduced to metallic gold under solvothermal conditions. Herein, we present the first example of Au-MOFs prepared from the networking of cyclic trinuclear gold(I) complexes by formal transimination reaction in a rapid (<15 min) and scalable (up to 1 g) fashion under ambient condition. The Au-MOFs feature uniform porosity, high crystallinity, and superior chemical stability toward base (i.e., 20 M NaOH). With open Au(I) sites in the skeleton, the Au-MOFs as heterogeneous catalysts delivered good performance and substrate tolerance for the carboxylation reactions of alkynes with CO2. This work demonstrates a facile approach to reticularly synthesize Au-MOFs by combining the coordination and dynamic covalent chemistry." @default.
• W4387325892 created "2023-10-05" @default.
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• W4387325892 date "2023-10-04" @default.
• W4387325892 modified "2023-10-14" @default.
• W4387325892 title "Gold(I)-Organic Frameworks as Catalysts for Carboxylation of Alkynes with CO₂" @default.
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• W4387325892 doi "https://doi.org/10.1021/jacs.3c08262" @default.
• W4387325892 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37791919" @default.
• W4387325892 hasPublicationYear "2023" @default.
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