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- W4387331410 abstract "Commercialization of photoelectrochemical (PEC) water‐splitting devices requires the development of large‐area, low‐cost photoanodes with high efficiency and photostability. Herein, we address these challenges by using scalable fabrication techniques and porous transport layer (PTLs) electrode supports. We demonstrate the deposition of W‐doped BiVO4 on Ti PTLs using successive‐ionic‐layer‐adsorption‐and‐reaction methods followed by boron treatment and chemical bath deposition of NiFeOOH co‐catalyst. The use of PTLs that facilitate efficient mass and charge transfer, allowed the scaling of the photoanodes (100 cm2) while maintaining ~90% of the performance obtained with 1 cm2 photoanodes for oxygen evolution reaction i.e. 2.10 mA cm‐2 at 1.23 V vs. RHE. This is the highest reported performance to date. Integration with a polycrystalline Si PV cell leads to bias‐free water splitting with a stable photocurrent of 208 mA for 6 h and 2.2% solar‐to‐hydrogen efficiency. Our findings highlight the importance of photoelectrode design towards scalable PEC device development." @default.
- W4387331410 created "2023-10-05" @default.
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- W4387331410 date "2023-10-04" @default.
- W4387331410 modified "2023-10-06" @default.
- W4387331410 title "Scaling up BiVO4 Photoanodes on Ti Porous Transport Layers for Solar Hydrogen Production" @default.
- W4387331410 doi "https://doi.org/10.1002/cssc.202300969" @default.
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