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- W4387342172 abstract "High-entropy materials (HEMs) represent a new class of solid solutions containing at least five different elements. Their compositional diversity makes them promising as platforms for the development of functional materials. We synthesized new HEMs in a mullite-type structure and present five compounds, i.e., Bi2(Al0.25Ga0.25Fe0.25Mn0.25)4O9 and A2Mn4O10 with variations of A = Nd, Sm, Y, Er, Eu, Ce, and Bi, demonstrating the vast accessible composition space. By combining scattering, microscopy, and spectroscopy techniques, we show that our materials are mixed solid solutions. Remarkably, when following their crystallization in situ using X-ray diffraction and X-ray absorption spectroscopy, we find that the HEMs form through a metastable amorphous phase without the formation of any crystalline intermediates. We expect that our synthesis is excellently suited to synthesizing diverse HEMs and therefore will have a significant impact on their future exploration." @default.
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- W4387342172 date "2023-10-04" @default.
- W4387342172 modified "2023-10-15" @default.
- W4387342172 title "High-Entropy Oxides in the Mullite-Type Structure" @default.
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- W4387342172 doi "https://doi.org/10.1021/acs.chemmater.3c01830" @default.
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