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- W4387402227 abstract "Abstract Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS 2 ) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS 2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS 2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling and important for practical optoelectronic devices based on low-dimensional semiconductors." @default.
- W4387402227 created "2023-10-07" @default.
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- W4387402227 date "2023-10-06" @default.
- W4387402227 modified "2023-10-17" @default.
- W4387402227 title "Ultrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature" @default.
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- W4387402227 doi "https://doi.org/10.21203/rs.3.rs-3409617/v1" @default.
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