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• W4387425552 endingPage "233675" @default.
• W4387425552 startingPage "233675" @default.
• W4387425552 abstract "A promising candidate for next-generation energy storage is the lithium-sulfur battery (LSB) due to its high capacity and low-cost active material (sulfur). However, the practical application of LSBs is challenged by poor cycling life and low sulfur loading. Herein, a proof-of-concept for manufacturing high load electrodes with a low-cost dry (solvent-free) coating process with a reduced carbon footprint is introduced and investigated. This process is often based on fluoropolymer-based binder additives with health and environmental concerns. Therefore, this study presents the concept of a binder-free dry coating process using sulfur/carbon black (S/CB) composites derived from a straight-forward dispersive mixing process. The electrodes are fabricated by a hot-pressing process, taking advantage of sulfur melting into a carbon matrix. To determine the process-structure-property relationships of the resulting powders, electrodes and cells, a novel structure determination by thermogravimetric analysis was used. Mixing time turns out to be an important factor, which has a significant effect on the electrode performance. The cells assembled with electrodes (⁓4.5 mgS cm−2) made from optimized powder mixtures showed a high specific capacity of about 800 mAh gS−1, and a relatively improved C-rate capability." @default.
• W4387425552 created "2023-10-08" @default.
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• W4387425552 date "2023-12-01" @default.
• W4387425552 modified "2023-10-18" @default.
• W4387425552 title "A binder-free dry coating process for high sulfur loading cathodes of Li–S batteries: A proof-of-concept" @default.
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• W4387425552 doi "https://doi.org/10.1016/j.jpowsour.2023.233675" @default.
• W4387425552 hasPublicationYear "2023" @default.
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