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- W4387451203 abstract "Abstract The light-dark cycles created from Earth’s rotation helped in the emergence of extant cellular life that integrates evolved oscillatory networks to control circadian rhythms, cell division, metabolism and so forth. Out of equilibrium networks of organic chemical reactions with dynamic self-assembled structures that emerged from Darwin’s nutrient-rich warm pond played crucial roles in spawning the protolife under a fluctuating environmental condition. Construction of chemical networks from simple chemicals that can display emergent network dynamics can contribute to our understanding of complex behaviours from simple organic reactions. Here we have designed single amino acid/dipeptide based systems that could demonstrate multiple periodic changes of (dis) assembly under non-equilibrium conditions in closed system, importantly in the absence of evolved biocatalysts. The two-component based building block exploited pH driven non-covalent assembly and time-delayed accelerated catalysis from self-assembled state to install orthogonal feedback loops with a single batch of reactants. Modifications of these autonomous systems from purely synthetic molecules can enable the design of exceptional life-like materials and evolving systems with acute spatiotemporal control of properties." @default.
- W4387451203 created "2023-10-10" @default.
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- W4387451203 date "2023-10-09" @default.
- W4387451203 modified "2023-10-11" @default.
- W4387451203 title "Minimal catalytic assemblies can demonstrate periodic (dis)assembly cycles in a closed system utilizing feedback loops" @default.
- W4387451203 doi "https://doi.org/10.21203/rs.3.rs-1235376/v2" @default.
- W4387451203 hasPublicationYear "2023" @default.
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