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• W4387473367 startingPage "9285" @default.
• W4387473367 abstract "We study the effect of sodium chloride (NaCl) on the properties of the interface of water and the surfactant dodecyl sulfate (DS-) using heterodyne-detected vibrational sum-frequency generation spectroscopy. We find that the signal of the O-H stretch vibrations of oriented water molecules at the interface is highly nonlinearly dependent on the NaCl concentration. This nonlinear dependence is explained by a combination of screening of the electric field of surface-bound DS- ions pointing into the bulk and screening of the Coulomb repulsion between the headgroups of the DS- ions in the surface plane. The latter effect strongly increases the oriented water signal within a limited NaCl concentration range of 10-100 mM, indicating a two-dimensional hydrophobic collapse of the surfactant layer. The occurrence of collapse is supported by model calculations of the surface potential and surface surfactant density." @default.
• W4387473367 created "2023-10-11" @default.
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• W4387473367 date "2023-10-10" @default.
• W4387473367 modified "2023-10-16" @default.
• W4387473367 title "Observation of a Two-Dimensional Hydrophobic Collapse at the Surface of Water Using Heterodyne-Detected Surface Sum-Frequency Generation" @default.
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• W4387473367 doi "https://doi.org/10.1021/acs.jpclett.3c01530" @default.
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• W4387473367 hasPublicationYear "2023" @default.
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