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• W4387491623 abstract "Abstract We report on a new form of nanoscale carbon nitride in the shape of single layer half dome structures grown on the step edges of boron nitride sheets. The half dome structures are formed spontaneously at high temperature in high vacuum using Fe 2 O 3 capped with N(CH 3 ) 4 OH supported on BN sheets. During the combustion process the BN support, firstly, acted as a reducing agent for the transformation of the iron oxide in metallic iron, secondly, as a source of nitrogen that permitted the transformation of the organic capping agent in sp 1 CN chains linked with sp 2 CN domains. During the Ostwald ripening processes smaller nanoparticles migrates towards bigger nanoparticle, when the nanoparticles come across the step edges of few layer boron nitrides sheets the half dome structure is formed. The propensity of FeNPs to catalyse the formation of the half dome containing cyanopolyynes species has been shown for the first time. The coexistence of carbon nitride atoms in two well-defined hybridization states within the CN@HDS may offer functional features characteristic of carbyne and carbon nitride." @default.
• W4387491623 created "2023-10-11" @default.
• W4387491623 creator A5022450785 @default.
• W4387491623 date "2023-10-10" @default.
• W4387491623 modified "2023-10-16" @default.
• W4387491623 title "Half dome carbon nitride nanostructures" @default.
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• W4387491623 doi "https://doi.org/10.21203/rs.3.rs-3407756/v1" @default.
• W4387491623 hasPublicationYear "2023" @default.
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