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- W4387573989 abstract "Catalytic CO2 desorption from rich amine solution is a practical approach to reducing energy consumption for amine regeneration. In this study, for the first time, the catalytic effect of environmentally friendly, imidazole series ionic liquids ([Bmim]PF6, [Bmim]BF4, [Bmim]HSO4, [Bmim]NO3, [Bmim]CH3COOH, [Bmim]Cl, [Bmim]Br, and [Bmim]I) is evaluated in terms of CO2 desorption rate, amount of CO2 released, and heat duty. Overall, the [Bmim]PF6 catalyst shows excellent catalytic activity for CO2 desorption, increasing the quantity of CO2 released by 21.35% and reducing the relative heat duty by 17.59%. In addition, the catalytic applicability of [Bmim]PF6 for secondary and tertiary amine systems was evaluated. Of note, the homogeneous [Bmim]PF6 catalyst presents good stability during 5 cycles. The catalyst/MEA (monoethanolamine) solution ratio of 3 wt% retained about 94% of the catalytic performance after five cycling tests without any reactivation step, showing the potential application of this desorption technology for CO2 capture with lower heat duty." @default.
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- W4387573989 date "2024-01-01" @default.
- W4387573989 modified "2023-10-15" @default.
- W4387573989 title "Energy-efficient regeneration of amine-based solvent with environmentally friendly ionic liquid catalysts for CO2 capture" @default.
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- W4387573989 doi "https://doi.org/10.1016/j.ces.2023.119380" @default.
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