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- W4387592185 endingPage "102628" @default.
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- W4387592185 abstract "The CALPHAD framework rests on the ability to assign well-defined free energies to all phases, including mechanically unstable ones. Given the experimental difficulties associated with the latter, researchers have turned to computational methods to obtain a theoretically justified definition of the free energy of mechanically unstable phases. Recently, a method called “inflection detection” has been shown to yield free energies that are broadly consistent with the current SGTE (Scientific Group Thermodata Europe) standard for pure elements, which were obtained through an extrapolation of stable solid solutions free energies towards unstable end members. Despite this general agreement, apparent failures for a few elements stand out, notably for the bcc–fcc enthalpy difference for the common element Al. Here we revisit the definition of the bcc Al enthalpy and show that a careful CALPHAD-based analysis of enthalpy trends in five different mechanically stable binary solid solutions in fact does agree very well with the inflection-detection approach." @default.
- W4387592185 created "2023-10-13" @default.
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- W4387592185 date "2023-12-01" @default.
- W4387592185 modified "2023-10-18" @default.
- W4387592185 title "Revisiting the SGTE lattice stability of bcc aluminum" @default.
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- W4387592185 doi "https://doi.org/10.1016/j.calphad.2023.102628" @default.
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