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- W4387595969 abstract "Combining the synthetic tunability of molecular compounds with the optical selection rules of transition metal dichalcogenides (TMDC) that derive from spin-valley coupling could provide interesting opportunities for the readout of quantum information. However, little is known about the electronic and spin interactions at such interfaces and the influence on spin-valley relaxation. In this work we investigate various heterojunctions of vanadyl phthalocyanine (VOPc) thermally evaporated on WSe$_2$ and find that local ordering of the molecular layer plays an important role in the electronic perturbation of WSe$_2$, which in turn directly influences the spin-valley polarization lifetime. A thin molecular layer results in a hybrid state which destroys the spin-valley polarization almost instantaneously, whereas a thicker molecular layer with well-defined local ordering shows minimal electronic perturbation and results in longer-lived spin-valley polarization than the WSe$_2$ monolayer alone." @default.
- W4387595969 created "2023-10-13" @default.
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- W4387595969 date "2023-10-10" @default.
- W4387595969 modified "2023-10-14" @default.
- W4387595969 title "Modulating Resonant Electronic Coupling of Tungsten Diselenide Monolayers with Vanadyl Phthalocyanine for Spin-Valley Polarization Control" @default.
- W4387595969 doi "https://doi.org/10.48550/arxiv.2310.06979" @default.
- W4387595969 hasPublicationYear "2023" @default.
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