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- W4387603517 abstract "Nanographenes are a class of extended π-conjugated molecules with great potential in photophysical and electrochemical properties. However, most nanographenes show self-aggregation due to their strong π–π interaction, resulting in struc-tures barely possessing any open π surface. We find that metal-organic frameworks (MOFs) can be an ideal platform to construct periodic arrays and pores with isolated large π-conjugated surfaces by avoiding undesired π–π interaction be-tween the nanographene molecules. Here, we report a multivariate series of nanographene-based MOFs, UMOF-2-X, utiliz-ing the graphene-like hexatopic organic linkers, hexaphenylbenzene (HPB) and hexabenzocoronene (HBC) through a mixed-linker strategy. Interestingly, UMOF-2 shows effective energy transfer between HPB and HBC linkers while sup-pressing the occurrence of linker-to-metal charge transfer from the linker to Cu metal. We successfully describe the origin of these intriguing phenomena through computational studies." @default.
- W4387603517 created "2023-10-14" @default.
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- W4387603517 date "2023-10-13" @default.
- W4387603517 modified "2023-10-14" @default.
- W4387603517 title "Nanographene-based Metal-Organic Frameworks for Engineering Energy Transfer Pathways" @default.
- W4387603517 doi "https://doi.org/10.26434/chemrxiv-2023-tbfns" @default.
- W4387603517 hasPublicationYear "2023" @default.
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