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• W4387608840 abstract "Carbon dioxide (CO2), a valuable feedstock, can be reutilized as a hydrogen carrier by hydrogenating CO2 to formic acid (FA) and releasing hydrogen by FA dehydrogenation in a reversible manner. Notably, FA is liquid at room temperature and can be stored and transported considerably more safely than hydrogen gas. Herein, we extensively reviewed transition-metal-based molecular catalysts explored for reversible CO2 hydrogenation and FA dehydrogenation. This Review describes different approaches explored for carbon-neutral hydrogen storage and release by applying CO2 hydrogenation to FA/formate and the subsequent release of H2 by the dehydrogenation of FA over a wide range of molecular catalysts based on noble and non-noble metals. Emphasis is also placed on the specific catalyst-to-substrate interaction by highlighting the specific role of the catalyst in the CO2 hydrogenation–FA dehydrogenation pathway." @default.
• W4387608840 created "2023-10-14" @default.
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• W4387608840 date "2023-10-13" @default.
• W4387608840 modified "2023-10-14" @default.
• W4387608840 title "Recent Developments in Reversible CO₂ Hydrogenation and Formic Acid Dehydrogenation over Molecular Catalysts" @default.
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• W4387608840 doi "https://doi.org/10.1021/acsomega.3c05286" @default.
• W4387608840 hasPublicationYear "2023" @default.
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