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- W4387644015 abstract "Although water electrolysis is one of the most environmentally friendly methods for producing hydrogen (H2) and oxygen, designing robust non-noble electrocatalysts for overall water splitting remains a massive challenge. Modulating the morphology and chemical composition of non-noble-metal bifunctional electrocatalysts is an effective way to enhance catalytic activity in water electrolysis. Herein, a robust electrocatalyst with porous CoP4/Co4S3 microcubes rich in defects was synthesized through the phosphorylation and hydrothermal vulcanization of a Co–Co Prussian blue analog (Co–Co PBA). Given that the as-prepared CoP4/Co4S3 microcubes can provide additional active sites to accelerate electron transfer at the heterointerface, they exhibit enhanced catalytic activities in hydrogen and oxygen evolution reactions in 1.0 M KOH. When used as a bifunctional catalyst in a two-electrode electrolyzer, the micrucubesrequire a cell voltage of 1.67 V to achieve a current density of 10 mA cm−2 in 1.0 M KOH, indicating its potential as an efficient alkaline non-noble electrocatalyst for overall water splitting. This study provides a promising electrocatalyst for clean H2 energy production by modulating its morphology and chemical composition." @default.
- W4387644015 created "2023-10-15" @default.
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- W4387644015 date "2023-10-01" @default.
- W4387644015 modified "2023-10-15" @default.
- W4387644015 title "The defect-rich porous CoP4/Co4S3 microcubes as robust electrocatalyst for clean H2 energy production via alkaline overall water splitting" @default.
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- W4387644015 doi "https://doi.org/10.1016/j.apcata.2023.119461" @default.
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