Matches in SemOpenAlex for { <https://semopenalex.org/work/W4387669478> ?p ?o ?g. }
Showing items 1 to 95 of
95
with 100 items per page.
- W4387669478 abstract "It is an appealing approach to CO2 utilization through CO2 electroreduction (CO2ER) to ethanol at high current density; however, the commonly used Cu‐based catalysts cannot sustain large current during CO2ER despite their capability for ethanol production. Herein, we report that Ag+‐doped InSe nanosheets with Se vacancies can address this grand challenge in a membrane electrode assembly (MEA) electrolyzer. As revealed by our experimental characterization and theoretical calculation, the Ag+ doping, which can tailor the electronic structure of InSe while diversifying catalytically active sites, enables the formation of key reaction intermediates and their sequential evolution into ethanol. More importantly, such a material can well work for large‐current conditions in MEA electrolyzers with In2+ species stabilized via electron transfer from Ag to Se. Remarkably, in an MEA electrolyzer by coupling cathodic CO2ER with anodic oxygen evolution reaction (OER), the optimal catalyst exhibits an ethanol Faradaic efficiency of 68.7% and a partial current density of 186.6 mA cm−2 on the cathode with a full‐cell ethanol energy efficiency of 26.1% at 3.0 V. This work opens an avenue for large‐current production of ethanol from CO2 with high selectivity and energy efficiency by rationally designing electrocatalysts." @default.
- W4387669478 created "2023-10-17" @default.
- W4387669478 creator A5032469771 @default.
- W4387669478 creator A5035477427 @default.
- W4387669478 creator A5036290384 @default.
- W4387669478 creator A5049078993 @default.
- W4387669478 creator A5050282787 @default.
- W4387669478 creator A5075632263 @default.
- W4387669478 creator A5087717847 @default.
- W4387669478 date "2023-10-16" @default.
- W4387669478 modified "2023-10-17" @default.
- W4387669478 title "Ag+‐Doped InSe Nanosheets for Membrane Electrode Assembly Electrolyzer toward Large‐Current Electroreduction of CO2 to Ethanol" @default.
- W4387669478 doi "https://doi.org/10.1002/ange.202313646" @default.
- W4387669478 hasPublicationYear "2023" @default.
- W4387669478 type Work @default.
- W4387669478 citedByCount "0" @default.
- W4387669478 crossrefType "journal-article" @default.
- W4387669478 hasAuthorship W4387669478A5032469771 @default.
- W4387669478 hasAuthorship W4387669478A5035477427 @default.
- W4387669478 hasAuthorship W4387669478A5036290384 @default.
- W4387669478 hasAuthorship W4387669478A5049078993 @default.
- W4387669478 hasAuthorship W4387669478A5050282787 @default.
- W4387669478 hasAuthorship W4387669478A5075632263 @default.
- W4387669478 hasAuthorship W4387669478A5087717847 @default.
- W4387669478 hasBestOaLocation W43876694781 @default.
- W4387669478 hasConcept C121332964 @default.
- W4387669478 hasConcept C123669783 @default.
- W4387669478 hasConcept C127413603 @default.
- W4387669478 hasConcept C130349721 @default.
- W4387669478 hasConcept C135473242 @default.
- W4387669478 hasConcept C147789679 @default.
- W4387669478 hasConcept C161790260 @default.
- W4387669478 hasConcept C163127949 @default.
- W4387669478 hasConcept C171250308 @default.
- W4387669478 hasConcept C17525397 @default.
- W4387669478 hasConcept C178790620 @default.
- W4387669478 hasConcept C179104552 @default.
- W4387669478 hasConcept C185592680 @default.
- W4387669478 hasConcept C192562407 @default.
- W4387669478 hasConcept C207740977 @default.
- W4387669478 hasConcept C2780161600 @default.
- W4387669478 hasConcept C2780302529 @default.
- W4387669478 hasConcept C33989665 @default.
- W4387669478 hasConcept C42360764 @default.
- W4387669478 hasConcept C48256821 @default.
- W4387669478 hasConcept C49110097 @default.
- W4387669478 hasConcept C52859227 @default.
- W4387669478 hasConcept C62520636 @default.
- W4387669478 hasConcept C65183824 @default.
- W4387669478 hasConcept C68801617 @default.
- W4387669478 hasConcept C75473681 @default.
- W4387669478 hasConcept C89395315 @default.
- W4387669478 hasConceptScore W4387669478C121332964 @default.
- W4387669478 hasConceptScore W4387669478C123669783 @default.
- W4387669478 hasConceptScore W4387669478C127413603 @default.
- W4387669478 hasConceptScore W4387669478C130349721 @default.
- W4387669478 hasConceptScore W4387669478C135473242 @default.
- W4387669478 hasConceptScore W4387669478C147789679 @default.
- W4387669478 hasConceptScore W4387669478C161790260 @default.
- W4387669478 hasConceptScore W4387669478C163127949 @default.
- W4387669478 hasConceptScore W4387669478C171250308 @default.
- W4387669478 hasConceptScore W4387669478C17525397 @default.
- W4387669478 hasConceptScore W4387669478C178790620 @default.
- W4387669478 hasConceptScore W4387669478C179104552 @default.
- W4387669478 hasConceptScore W4387669478C185592680 @default.
- W4387669478 hasConceptScore W4387669478C192562407 @default.
- W4387669478 hasConceptScore W4387669478C207740977 @default.
- W4387669478 hasConceptScore W4387669478C2780161600 @default.
- W4387669478 hasConceptScore W4387669478C2780302529 @default.
- W4387669478 hasConceptScore W4387669478C33989665 @default.
- W4387669478 hasConceptScore W4387669478C42360764 @default.
- W4387669478 hasConceptScore W4387669478C48256821 @default.
- W4387669478 hasConceptScore W4387669478C49110097 @default.
- W4387669478 hasConceptScore W4387669478C52859227 @default.
- W4387669478 hasConceptScore W4387669478C62520636 @default.
- W4387669478 hasConceptScore W4387669478C65183824 @default.
- W4387669478 hasConceptScore W4387669478C68801617 @default.
- W4387669478 hasConceptScore W4387669478C75473681 @default.
- W4387669478 hasConceptScore W4387669478C89395315 @default.
- W4387669478 hasLocation W43876694781 @default.
- W4387669478 hasOpenAccess W4387669478 @default.
- W4387669478 hasPrimaryLocation W43876694781 @default.
- W4387669478 hasRelatedWork W2306864182 @default.
- W4387669478 hasRelatedWork W2517928179 @default.
- W4387669478 hasRelatedWork W3169220044 @default.
- W4387669478 hasRelatedWork W4200049192 @default.
- W4387669478 hasRelatedWork W4210441988 @default.
- W4387669478 hasRelatedWork W4303021529 @default.
- W4387669478 hasRelatedWork W4312193406 @default.
- W4387669478 hasRelatedWork W4313255878 @default.
- W4387669478 hasRelatedWork W4320018844 @default.
- W4387669478 hasRelatedWork W4322758744 @default.
- W4387669478 isParatext "false" @default.
- W4387669478 isRetracted "false" @default.
- W4387669478 workType "article" @default.