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- W4387675983 abstract "CO esterification to dimethyl oxalate (DMO) has important industrial application value. However, the influence of support on catalytic performance has not been investigated sufficiently. In this work, MgAl-LDO supports (MgAl-LDO-400 and MgAl-LDO-600) were prepared at different calcination temperatures. The corresponding Pd-based catalysts was synthesized by impregnation method. The Pd/MgAl-LDO-400 catalyst exhibited higher CO conversion (39%) compared with the Pd/MgAl-LDO-600 (16%). It was found that Pd/MgAl-LDO-400 catalyst contains more Lewis basic sites, which is responsible for its higher activity. This work provides a general understanding of the support effect on catalytic performance induced by the Lewis basic sites." @default.
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- W4387675983 date "2023-10-01" @default.
- W4387675983 modified "2023-10-17" @default.
- W4387675983 title "Enhanced catalytic activity for CO esterification to dimethyl oxalate via increasing Lewis basic sites in Pd/MgAl-LDO catalyst" @default.
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- W4387675983 doi "https://doi.org/10.1016/j.catcom.2023.106781" @default.
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