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- W4387676224 abstract "The onstruction of novel porous carbon materials for efficient desalination is crucial but remains challenging for capacitive deionization (CDI) development. Herein, a micelle-assisted strategy was raised to coat mesoporous polydopamine (mPDA) on the surface of two-dimensional (2D) leaf-like zeolitic imidazolate frameworks (ZIFL) followed by confinement pyrolysis. The introduction of the mPDA layer can not only mitigate the backbone collapse of ZIFL during pyrolysis to build a favorable porous environment for efficient ion transport and diffusion, but also induce explosive growth of carbon nanotubes (CNTs) to improve the electron conductivity. As excepted, the derivative ZIFL@mPDA-C possessed a high desalination capacity of 41.9 mg g−1 in 500 mg/L NaCl solution at an operating voltage of 1.2 V. In particular, the retention ratio of the desalination capacity of ZIFL@mPDA-C was about 100 % after 50 consecutive adsorption-desorption cycles, while its leaf-like morphology and hierarchical pore structures were well preserved. This study highlights the importance of rationally designed structures and components for the performance breakthrough of carbon-based CDI electrode materials." @default.
- W4387676224 created "2023-10-17" @default.
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- W4387676224 date "2023-10-01" @default.
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- W4387676224 title "Mesoporous dopamine-modified leaf-like zeolitic imidazolate frameworks derived carbon for efficient capacitive deionization" @default.
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- W4387676224 doi "https://doi.org/10.1016/j.jcis.2023.10.070" @default.
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