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- W43938600 abstract "A NO/sub 2/ absorption enhancement under conditions of water condensation may be that there is a net movement of water vapor toward the water surface, tending to drag extra NO/sub 2/ molecules along, whereas in the steady-state condition there exists an equimolar exchange of water molecules both to and from the surface. The results show that, as H/sub 2/O condensation ceases, the NO/sub 2/ concentration level rapidly returns to saturation. Mechanisms which may promote this phenomenon are: (a) as evaporation takes over the outer layers of solution are stripped away, releasing NO/sub 2/ back into the atmosphere; (b) dissolved NO/sub 2/, present either as NO/sub 2//sup -/ or NO/sub 3//sup -/ may become too concentrated in the outer layers and revert to NO/sub 2/ and then escape as a gas; (c) evaporating water molecules in the vicinity of the interface may reduce the gas phase NO/sub 2/ concentration to a level below that in the bulk gas, providing an extra driving force. The fact that the desorption is so rapid indicates that any one or a combination of the above mechanisms are acting more rapidly than the combined liquid phase diffusion-chemical reaction mechanism tending to absorb the NO/sub 2/ intomore » the droplet interior.« less" @default.
- W43938600 created "2016-06-24" @default.
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- W43938600 date "1977-01-01" @default.
- W43938600 modified "2023-09-27" @default.
- W43938600 title "Nitrogen dioxide absorption in evaporating and condensing water droplets" @default.
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