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- W44980510 abstract "Uni-, two-, and three-dimensional vibrational modes occur in spherical top molecules. Fundamental transitions are allowed only to three-dimensional vibrational states, and only the components of three-dimensional modes can be split by Coriolis coupling. The rotational structure of fundamental transitions involves the coupling of the vibrational and total angular momenta and is examined in the details. The rotational structure of overtones and combination states involving the multiple excitation of three-dimensional modes is also examined, and typical limit coupling representations are discussed, with account for the effects of anharmonicity. It is shown that a vibration-rotation manifold is close to a representation with defined angular momentum quantum numbers, if the coupling is dominated by the Coriolis and scalar anharmonic operators. A different coupling scheme, with well-defined vibrational symmetries, gives a better description of the system if the coupling is dominated by the tensor anharmonic terms." @default.
- W44980510 created "2016-06-24" @default.
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- W44980510 date "2013-01-01" @default.
- W44980510 modified "2023-09-24" @default.
- W44980510 title "Spectra of Spherical Top Molecules" @default.
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- W44980510 doi "https://doi.org/10.1016/b978-0-12-407771-3.00010-0" @default.
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