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- W45848650 abstract "A layer of magnetite identified from the Moessbauer spectrum on a steel surface in an acidic (pH 2-4), very weak solution of sodium nitrate grows in accordance with a parabolic law against the background of a steady flow of iron ions into solution. As shown by radioactive labeling, the ions are formed by the dissolution not of the oxide but of the underlying metal. Careful study shows that the dissolution is electrochemical and is limited by the diffusion supply of hydrogen ions. The special colloidal mechanism of formation of an ultraporous magnetite layer is based on mutual balancing of tendencies toward cathodic alkalization of the solution near the electrode and its acidification by the dissociation (hydrolysis) of aqueous complexes of Fe/sup 2 +/. An increase in temperature thermodynamically and kinetically intensifies the formation of the oxide. A preliminary model of this neglected mechanism is given." @default.
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- W45848650 date "1987-11-01" @default.
- W45848650 modified "2023-09-26" @default.
- W45848650 title "Colloidal-electrochemical mechanism of oxidative corrosion of steel in hot nitrate-containing water" @default.
- W45848650 hasPublicationYear "1987" @default.
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