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- W47410614 abstract "Lacking the symmetric order of solids or the isolation of gases, liquids are intrinsically more complicated than the other states of matter due to the inherent randomness and the subtle interplay of various many-body interactions. In understanding the dynamics of liquids in chemical processes, it is sensible to look first at dynamics of pure liquids. The timescales, on which interesting phenomena occur, span many orders of magnitude, but the basic interactions are fundamentally determined by vibrational periods, and these are generally sub-picosecond. Liquids motions are characterized by frequencies that are smaller than typical intramolecular bond vibrations, and are generally in the range from 10-500 cm -1 . Though tremendous recent progress has been made in the study of intramolecular vibrations, their couplings and even hydrogen bonded systems, these approaches yield only a local picture of the liquid. To build a picture of a solvent, one needs to focus on the larger scale dynamics involving many solvent molecules, and direct the attention towards collective dynamics. However, this is a conceptually challenging prospect that places significant demands on the state of the art of both theoretical descriptions and experimental techniques." @default.
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- W47410614 date "2004-01-01" @default.
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- W47410614 title "Femtosecond liquid dynamics studied by two-dimensional Raman spectroscopy" @default.
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- W47410614 doi "https://doi.org/10.1016/b978-044451656-5/50054-2" @default.
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