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- W4917812 abstract "In recent years, there has been a considerable commercial interest in the Fischer-Tropsch (FT) reaction, which converts syngas to liquid products. Partial oxidation of methane (POM) is energy efficient and is expected to produce syngas with a H 2 /CO ratio of about 2, which is suitable for Gas-to-Liquids (GTL) technology. In this study, the performance of catalytic methane oxidation reactions in a small channel plate reactor has been investigated. The main advantage of catalytic plate reactors over conventional ones is the negligible intra-catalyst diffusion resistance. For plate reactors to be successful, the catalyst must have a high activity and long life. Thin layers of catalyst (≤ 50 μm) prepared using a sol-gel method showed some promise for achieving this objective. POM reactions were investigated in the small channels coated by thin film catalyst. The results showed that methane-air mixtures can efficiently be converted into synthesis gas (H 2 /CO ratio ≈ 2) at temperatures higher than 800 °C. It has been shown that the stability and coking resistance of Ni/Al 2 O 3 catalyst are increased by addition of Ba, Cr and La 2 O 3 in partial oxidation of methane. This work has demonstrated the potential advantages of plate reactor over conventional types of reactors; neither hot spots nor thermal runaway were observed during methane partial oxidation reactions. The values of activation energy indicate that the POM reaction is free from any diffusion limitation effect. It has been established that sol gel method facilitates the catalyst preparation. The sol-gels can be prepared to have desirable rheological properties for coating onto stainless steel substrates, which after calcining form an adherent thin catalyst layer." @default.
- W4917812 created "2016-06-24" @default.
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- W4917812 date "2009-01-01" @default.
- W4917812 modified "2023-09-23" @default.
- W4917812 title "GTL Feed by Catalytic Oxidation of Methane in Plate Reactor" @default.
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- W4917812 doi "https://doi.org/10.1016/b978-0-444-53292-3.50044-4" @default.
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