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- W51069011 abstract "The reduction of Pu(IV) using photochemically generated U(IV) has been evaluated as a procedure for possible inclusion in the Savannah River Plant's nuclear fuel reprocessing facility. The ''Purex 2nd Uranium Cycle'' with feed conditions of 400 g/L U, 1 M HNO/sub 3/, and 10/sup -8/ to 10/sup -6/ M Pu was identified previously as the most promising stage for application of a photochemical method. Laboratory tests were conducted under similar conditions to determine if the plutonium could be successfully reduced and separated in a two-phase flowing system. The laboratory scale tests, which used primarily a 0.01 M butanol/0.01 M hydrazine reductant combination, demonstrated that reductive stripping of Pu(IV) using photochemically generated U(IV) is a practical method for removing plutonium from the organic phase. The kinetics of the reductive stripping procedure were found to be determined by the mixing rates of the organic and aqueous phases in this simple laboratory-scale system." @default.
- W51069011 created "2016-06-24" @default.
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- W51069011 date "1986-05-01" @default.
- W51069011 modified "2023-09-24" @default.
- W51069011 title "Reduction of plutonium(IV) using photochemically generated uranium(IV)" @default.
- W51069011 doi "https://doi.org/10.2172/5813648" @default.
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