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- W54926311 abstract "Water-soluble palladium complexes of the sodium salt of trisulfonated triphenylphosphine (tppts, P(C6H4-m-SO3Na)3) catalyze the aqueous biphasic hydrocarboxylation of olefins. High catalytic activities were observed with small, sparingly water-soluble olefins such as propene (TOF>2800 h−1 in the conversion to n- and isobutyric acid). Although selectivities (n/iso ratio) were rather moderate in the hydrocarboxylation of propene and 1-octene, high selectivities (>99%) were observed in the conversion of isobutene or cyclopentene to 3-methylbutyric acid and cyclopentanecarboxylic acid, respectively. The water-soluble Pd catalyst based on the bidentate phosphine dpppr-s (1,3-C3H6(P(C6H4-m-SO3Na)2)2) catalyzes the alternating copolymerization of CO and olefins to polyketones. Activities >4.0 kg of copolymer per gram Pd per hour were found in the alternating copolymerization of CO and ethene." @default.
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- W54926311 date "1999-10-01" @default.
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- W54926311 title "Catalytic conversions in water" @default.
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- W54926311 doi "https://doi.org/10.1016/s1381-1169(99)00065-5" @default.
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