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- W5591217 abstract "Abstract The state of a catalyst surface on which the main reaction and the coking reaction occur simultaneously is described rigorously, based upon a stochastic approach. This approach, combined with a Boolean reaction matrix, has the advantage that it lends itself to solving complex reaction mechanisms because the RHS of the governing stiff differential equations can easily be generated by computer. Several reaction schemes have been explored and confirm results obtained by a less general model proposed by Nam and Froment (1987). When all reaction steps require only one site to proceed, the system belongs to the class of structure-insensitive reactions. When all or some reaction steps require more than one site, the system can become structure sensitive. The influence of the site coverage on the selectivity for the main reaction in a more complex reaction and the optimization of the cluster size are also illustrated." @default.
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- W5591217 date "1987-01-01" @default.
- W5591217 modified "2023-10-07" @default.
- W5591217 title "Stochastic Modeling of Catalyst Deactivation by Site Coverage." @default.
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- W5591217 doi "https://doi.org/10.1016/s0167-2991(09)60374-8" @default.
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