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- W58365057 abstract "The hybrid and sulfur-iodine (SI) thermochemical processes are the leading candidates worldwide for production of hydrogen (H2) using nuclear energy. In both processes, water plus high-temperature heat yields hydrogen and oxygen. In each process there is a series of chemical reactions in which all the chemicals, with the exception of water, are recycled. The processes are potentially efficient, scalable to large sizes, and economic. However, both processes have one major disadvantage: high operating temperatures (800 to 900°C). Both processes have the same hightemperature steps: the equilibrium thermal decomposition of sulfuric acid into H2O, O2, and SO3 followed by the decomposition of SO3 into O2 and SO2. The high temperatures are at the limits of materials of construction for heat exchangers and other components. The peak reaction temperatures can be lowered by ~200°C if the high-temperature decomposition products of sulfuric acid (O2, H2O, and SO2) can be separated from SO3 as they are formed. Selective separation of reaction products allows the reaction to be driven to completion at lower temperatures. Experiments are under way at Oak Ridge National Laboratory to develop an inorganic membrane to accomplish this task. The preliminary data on the separation of O2 and SO2 from SO3 using an inorganic membrane are reported." @default.
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- W58365057 date "2004-01-01" @default.
- W58365057 modified "2023-09-24" @default.
- W58365057 title "Sulfur Thermochemical Processes with Inorganic Membranes to Produce Hydrogen" @default.
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