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• W607454988 abstract "We reinvestigate the applicability of the concept of trap-free carrier transport in molecularly doped polymers and the possibility of realistically describing time-of-flight (TOF) current transients in these materials using the classical convection–diffusion equation (CDE). The problem is treated as rigorously as possible using boundary conditions appropriate to conventional time of flight experiments. Two types of pulsed carrier generation are considered. In addition to the traditional case of surface excitation, we also consider the case where carrier generation is spatially uniform. In our analysis, the front electrode is treated as a reflecting boundary, while the counter electrode is assumed to act either as a neutral contact (not disturbing the current flow) or as an absorbing boundary at which the carrier concentration vanishes. As expected, at low fields transient currents exhibit unusual behavior, as diffusion currents overwhelm drift currents to such an extent that it becomes impossible to determine transit times (and hence, carrier mobilities). At high fields, computed transients are more like those typically observed, with well-defined plateaus and sharp transit times. Careful analysis, however, reveals that the non-dispersive picture, and predictions of the CDE contradict both experiment and existing disorder-based theories in important ways, and that the CDE should be applied rather cautiously, and even then only for engineering purposes." @default.
• W607454988 created "2016-06-24" @default.
• W607454988 creator A5008279943 @default.
• W607454988 creator A5026105452 @default.
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• W607454988 date "2015-08-01" @default.
• W607454988 modified "2023-09-24" @default.
• W607454988 title "Non-dispersive carrier transport in molecularly doped polymers and the convection–diffusion equation" @default.
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• W607454988 doi "https://doi.org/10.1016/j.chemphys.2015.06.001" @default.
• W607454988 hasPublicationYear "2015" @default.
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