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• W620725423 abstract "This work demonstrates the feasibility of measuring electrochemical reaction rates on common flow-through porous electrodes by traditional Tafel analysis. A customized microfluidic channel electrode was designed and demonstrated by measuring the intrinsic kinetics of the V2 +/V3 + and VO2 +/VO2+ redox reactions in carbon paper electrodes under forced electrolyte flow. The exchange current density of the V2 +/V3 + reaction was found to be nearly two orders of magnitude slower than the VO2 +/VO2+ reaction, indicating that this may be the limiting reaction in vanadium redox flow batteries. The forced convection in this technique is found to generate reproducible exchange current densities which are consistently higher than for conventional electrochemical methods due to improved mass transport." @default.
• W620725423 created "2016-06-24" @default.
• W620725423 creator A5021136042 @default.
• W620725423 creator A5054676737 @default.
• W620725423 creator A5056229295 @default.
• W620725423 date "2015-08-01" @default.
• W620725423 modified "2023-10-17" @default.
• W620725423 title "Direct measurement of electrochemical reaction kinetics in flow-through porous electrodes" @default.
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• W620725423 doi "https://doi.org/10.1016/j.elecom.2015.04.019" @default.
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