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- W63452035 abstract "An absorption-cell technique is utilized to determine the rate constants for the C${mathrm{O}}_{2}$ ${02}^{0}$0-${10}^{0}$0 relaxation in C${mathrm{O}}_{2}$ and binary-gas mixtures of C${mathrm{O}}_{2}$-He and C${mathrm{O}}_{2}$-${mathrm{N}}_{2}$. The experiment consists of injecting a ensuremath{sim}2-nsec 10.4-ensuremath{mu}m pulse through the absorption cell---saturating the C${mathrm{O}}_{2}$ ${10}^{0}$0 to ${00}^{0}$1 transition, and monitoring the subsequent molecular re-equilibrations by recording the temporal intensity of a spatially overlapping probe beam in the 9.4-ensuremath{mu}m band connecting the ${02}^{0}$0 and ${00}^{0}$1 states. The measured rate constants are ${k}_{mathrm{C}{mathrm{O}}_{2}ensuremath{-}mathrm{C}{mathrm{O}}_{2}}=3ifmmodepmelsetextpmfi{}1$, ${k}_{mathrm{C}{mathrm{O}}_{2}ensuremath{-}mathrm{He}}=0.8ifmmodepmelsetextpmfi{}0.3$, and ${k}_{mathrm{C}{mathrm{O}}_{2}ensuremath{-}{mathrm{N}}_{2}}=3ifmmodepmelsetextpmfi{}1$, all in units of ${10}^{5}$ ${mathrm{sec}}^{ensuremath{-}1}$ ${mathrm{Torr}}^{ensuremath{-}1}$. The experimental approach also yields information on the thermalization of other processes having slower rates, and these are discussed qualitatively. Finally, a comparison is made with other related experimental investigations and two calculations which predict values for ${k}_{mathrm{C}{mathrm{O}}_{2}ensuremath{-}mathrm{C}{mathrm{O}}_{2}}$ appreciably different from those measured." @default.
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- W63452035 title "Rate constants for the C<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>O</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math><mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:mrow><mml:mn>02</mml:mn></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math>0-<mml:math xmlns:mml=http://www.w3.org/…" @default.
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- W63452035 doi "https://doi.org/10.1103/physreva.11.54" @default.
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