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- W66414037 abstract "A collaborative study between two laboratories was undertaken to determine Fischer-Tropsch activity and selectivity properties of representative cobalt and iron catalysts under conditions relevant to natural-gas to liquids conversion. In FTS activity/selectivity tests of Co/Al2O3 and Fe/K/Cu supported on silica, conducted under comparable operating conditions, i.e., H2/CO = 2, Ptot = 20 bar, GHSV = 2.1 NL/gcat/h and 50-70% CO conversion, 20-25% higher catalyst-mass-based CO conversion activity is observed for CO/Al2O3 relative to Fe/K/Cu/Si. Site-based rates (i.e., turnover frequencies based on H2 chemisorption data) are two times higher for Co/Al2O3 relative to Fe/K/Cu/Si. C5 + selectivity for Co/Al2O3 is 50-60% higher due to its higher propagation probability and its negligible CO2 selectivity; its C2 + productivity is also 50-70% higher because of its higher activity and higher selectivity to C2 + hydrocarbons. Activity and selectivity data obtained in the laboratories of Brigham Young University and EniTecnologie using micro and bench scale fixed bed reactors are in the case of Co/Al2O3 in excellent agreement and in the case of Fe/K/Cu/Si in fairly good agreement." @default.
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- W66414037 date "2001-01-01" @default.
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- W66414037 title "Quantitative Comparison of Supported Cobalt and Iron Fischer Tropsch Synthesis Catalysts" @default.
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- W66414037 doi "https://doi.org/10.1016/s0167-2991(01)80355-4" @default.
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