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- W756786564 abstract "Bisphenol A (BPA) is a ubiquitous environmental contaminant with endocrine disruption potential. This study explored the efficiency, kinetics, and mechanism of BPA removal from weakly acidic solutions by using NaBiO3 as a source of singlet oxygen. It was observed that the use of NaBiO3 (1gL(-1)) could eliminate almost all (more than 97%) of the added BPA (0.1mmolL(-1)) in solutions at pH 5.0 in 60min. The degradation of BPA followed pseudo-first-order kinetics over the pH range from 3 to 9, and the pseudo-first-order rate constant (k) was dependent on pH, NaBiO3 concentration and the coexisting compounds. As solution pH was decreased from 9 to 3 or NaBiO3 concentration was increased from 0.5 to 2gL(-1), the k value was increased logarithmically. Humic acid and Fe(3+) showed little effect on the BPA removal, but Mn(2+) exhibited exceptionally enhancing effect on the degradation of BPA. The involved reactive species were identified as singlet oxygen by using radical scavenger probes and ESR measurement, and the generated singlet oxygen was confirmed to be generated from the decomposition of NaBiO3 mediated by H(+) ions." @default.
- W756786564 created "2016-06-24" @default.
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- W756786564 date "2015-12-01" @default.
- W756786564 modified "2023-10-14" @default.
- W756786564 title "In situ H + -mediated formation of singlet oxygen from NaBiO 3 for oxidative degradation of bisphenol A without light irradiation: Efficiency, kinetics, and mechanism" @default.
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- W756786564 doi "https://doi.org/10.1016/j.chemosphere.2015.06.048" @default.
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