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- W78609106 abstract "Portland cements are commercially available construction materials that contain high concentrations of calcium silicates. The silicates are highly reactive towards SO/sub 2/ at temperatures and pressures encountered in atmospheric and pressurized FBC's. Of the Portland cements tested, PC III appears to have the highest sulfation capacity when sulfated by SO/sub 2/ at FBC conditions. A thermodynamic analysis of the sulfation of calcium silicates indicates that they are capable of reducing the concentration of SO/sub 2/ in FBC combustion gases to within the current EPA emission limits. The optimum temperature for sulfation of 16/20 mesh PC III pellets is about 1000/sup 0/C in comparison to about 875/sup 0/ for natural limestones. The higher observed optimum temperature is an advantage because combustion and power cycle efficiencies tend to increase as bed temperature increases. The reactions for regenerating sulfated calcium silicates are similar to those for regenerating calcium sulfate. However, the equilibrium partial pressures of SO/sub 2/ in the reductive decomposition of sulfated silicates are much higher than for sulfate lime. This implies that higher SO/sub 2/ concentrations will be attainable in the regenerator off-gas which will result in more economical conversion of SO/sub 2/ to sulfur or sulfuric acid. The sulfation capacity more » and regeneration efficiency of PC III pellets do not deteriorate with repeated sulfation/regeneration cycling. This indicates that PC III pellets are suitable for use in regenerative systems. The sulfation capacity of PC III is independent of pressure up to at least 10 atm. « less" @default.
- W78609106 created "2016-06-24" @default.
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- W78609106 date "1980-01-01" @default.
- W78609106 modified "2023-09-26" @default.
- W78609106 title "Regenerative Portland cement sorbents for fluidized-bed combustion of coal" @default.
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