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- W791257548 abstract "The advent of picosecond (ps) [1,2] and more recently the first femtosecond (fs) [3] laser pulses now offers access to a time regime in simple liquids which approaches an interval corresponding perhaps to less than one hundred collisions. Yet, within this period, intermolecular potentials are sensitive to local density and configurational fluctuations, and the molecular dynamics to spatial correlations, which may persist over hundreds of collisions. This is the glimpse of memory in liquids. To what extent the early time behaviour of a molecular system at liquid densities can be adequately described by hydrodynamic models, developed from generalised Langevin equations, or by kinetically motivated models emphasizing collisional behaviour, has been a topic of considerable theoretical interest[4] in recent years and a long standing goal of our research in picosecond and nonlinear laser spectroscopy[5]. However, because the temporal profile of the laser pulse is often of finite width with respect to the time-evolution of the molecular response and its decay, the properties of the pump and probe laser pulses become a significant and even deterministic part of the problem when exploring such memory in liquids." @default.
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- W791257548 date "1982-01-01" @default.
- W791257548 modified "2023-09-27" @default.
- W791257548 title "Subpicosecond Laser Spectroscopy: Pulse Diagnostics and Molecular Dynamics in Liquids" @default.
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- W791257548 doi "https://doi.org/10.1007/978-3-642-87864-0_55" @default.
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