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- W791466444 abstract "The diffusion controlled reaction of oxygen with films of bituminous binders is the main cause of the (long-term) hardening of bitumens in pavement surfacings. Earlier work on this reaction was confined to studies of the initial reaction rate and the analytical solution for the differential equation which describes the steady state of the system. A finite difference method to evaluate the equation for the unsteady state had been developed so that the effects of extended reaction times could be studied. The reaction was assumed to be retarded by exhaustion of reactive constituents in the binder and by the reaction products increasing binder viscosity and reducing the rate of diffusion of oxygen through it. The effect of binder reactivity, temperature and length of diffusion path were examined, and it was calculated that long-term binder hardening will be very slow at locations in a bituminous construction where the diffusion path through the binder from a surface exposed to air exceeds about 3 mm. More information is needed on the relationship between the amount of oxygen reacting with a binder and the increase of viscosity which this reaction produces before the system can be more precisely defined. (Author/TRRL)" @default.
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- W791466444 date "1984-09-01" @default.
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- W791466444 title "THE DIFFUSION CONTROLLED REACTION OF OXYGEN WITH FILMS OF BITUMINOUS BINDERS" @default.
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