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- W84656197 abstract "Gamma radiolysis of polycrystalline djenkolic acid at room temperature produces two groups of carbon radicals. The radicals of group A either decay by a second-order reaction or are converted to sulfur radicals by a pseudo first-order process, while the radicals of group B can only be converted to sulfur radicals. The carbon radicals of groups A and B appear to be the same chemical species but differ in their microenvironments. Addition of ${rm Co}^{2+}, {rm Ni}^{2+}$, and Fe2+ at a ratio of 1 metal ion per 10 molecules of djenkolic acid decreases the initial yield of carbon radicals and increases the second-order decay rate and the percentage of carbon radicals belonging to group A. Addition of ${rm Na}_{2}{rm SO}_{4}, {rm NaNO}_{3},{rm CdSO}_{4}$, and ${rm Ni}^{2+}-{rm EDTA}$ has no effect. The second-order decay may be explained by a vacancy-controlled bulk-diffusion process; metal ions appear to exert their influence by increasing the number of lattice defects. Addition of certain metals, pa..." @default.
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- W84656197 date "1974-05-01" @default.
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- W84656197 title "Effects of Metal Ions on the γ-Radiolysis of Polycrystalline Djenkolic Acid" @default.
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- W84656197 doi "https://doi.org/10.2307/3573928" @default.
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