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- W848202328 abstract "Incorporation of redox non-innocent ligands as well as pendant acid/base moieties has proven effective as a method for overcoming the propensity for earth-abundant transition metals to preferentially access single-electron chem. and facilitate efficient multi-proton, multi-electron activation of small mols. such as dioxygen. A series of molybdenum-quionoid complexes supported by a non-innocent ligand have been synthesized and characterized demonstrating both hydrogen atom and proton and electron transfer chem. spanning a total of four electrons and two protons. Five different protonation/oxidn. state combinations were isolated varying from Mo(0)-catechol to Mo(II)-quinone. Substrate-based multi-proton, multi-electron reactivity was demonstrated through redn. of dioxygen to water, and mechanistic insight gained via substituting the protons for other Lewis-acidic moieties will also be presented." @default.
- W848202328 created "2016-06-24" @default.
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- W848202328 date "2014-08-01" @default.
- W848202328 modified "2023-09-27" @default.
- W848202328 title "Synthesis, characterization, and multi-proton/multi-electron chemistry of molybdenum-quinoid complexes supported by a non-innocent ligand" @default.
- W848202328 hasPublicationYear "2014" @default.
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