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- W87085621 abstract "The theory of the multi-vibrational electron transitions based on the adiabatic representation for the wave functions of the initial and final states is the subject of this chapter. Then, the matrix element for radiationless multi-vibrational electron transition is the product of the electron matrix element and the nuclear element. The presented theory is devoted to the calculation of the nuclear component of the transition probability. The different calculation methods developed in the pioneer works of S.I. Pekar, Huang Kun and A. Rhys, M. Lax, R. Kubo and Y. Toyozawa will be described including the operator method, the method of the moments, and density matrix method. In the description of the high-temperature limit of the general formula for the rate constant, specifically Marcus's formula, the concept of reorganization energy is introduced. The application of the theory to electron transfer reactions in polar media is described. Finally, the adiabatic transitions are discussed." @default.
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- W87085621 date "2007-01-01" @default.
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- W87085621 title "Chapter 2 Conventional Theory of Multi-Phonon Electron Transitions" @default.
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- W87085621 doi "https://doi.org/10.1016/s1079-4050(06)34002-1" @default.
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