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- W88755899 endingPage "3438" @default.
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- W88755899 abstract "The interaction of Ti${mathrm{O}}_{2}$(110) with ${mathrm{O}}_{2}$, ${mathrm{H}}_{2}$, CO, and C${mathrm{O}}_{2}$ was studied by means of low-energy electron diffraction, x-ray photoelectron spectroscopy, electron energy-loss spectroscopy, thermal desorption, electron paramagnetic resonance, and measurements of changes in surface conductivities, $ensuremath{Delta}ensuremath{sigma}$, and work functions, $ensuremath{Delta}ensuremath{phi}$, for $300ensuremath{le}Tensuremath{le}1000$ K with particular emphasis on surface reactions involving intrinsic surface defects $2{mathrm{Ti}}^{3+}ifmmodecdotelsetextperiodcenteredfi{}V_{O}^{}{}_{}{}^{(+)}$. The defects are thermodynamically stable at high temperatures and act as donors and specific adsorption sites for ${mathrm{H}}_{2}$ and CO. Surface and subsurface reactions involving ${mathrm{O}}_{2}$, ${mathrm{H}}_{2}$, CO, and C${mathrm{O}}_{2}$ can be separated from each other by analyzing the $ensuremath{Delta}ensuremath{sigma}$ and $ensuremath{Delta}ensuremath{phi}$ effects in a charge-transfer model, which takes into account surface and bulk electronic states in the band gap attributed to the different defects formed during the interaction." @default.
- W88755899 created "2016-06-24" @default.
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- W88755899 creator A5029798447 @default.
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- W88755899 date "1983-09-15" @default.
- W88755899 modified "2023-10-17" @default.
- W88755899 title "Intrinsic defects of Ti<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>O</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>(110): Interaction with chemisorbed<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>O</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow…" @default.
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- W88755899 doi "https://doi.org/10.1103/physrevb.28.3427" @default.
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