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- W90171716 abstract "Removal of nitrogen oxides and fission product iodine from the offgas generated by dissolution is essential in the reprocessing of spent nuclear reactor fuel. The species NO, NO/sub 2/, N/sub 2/O/sub 3/, and N/sub 2/O/sub 4/ can account for as much as ten percent or the offgas generated by the dissolution of mixed oxide (Pu-O) fuels in nitric acid. While the radioisotopes of iodine are present in much smaller concentrations (only 15 grams are evolved in the dissolution of 500 Kg of 180-day cooled spent fuel), the radiological hazards it posses make the containment, partitioning, and disposal of iodine of paramount importance. A computer simulation which combines NO/sub x/ scrubbing with iodine liquidvapor partitioning and hydrolysis has been developed and used to evaluate a number of possible offgas system flowsheets. The conclusions reached using this simulation agree closely with experimentally obtained data. A generalized conclusion drawn from this study is that flowsheets which provide optimal processing of either NO/sub x/ or iodine do not provide optimal removal or both components. Therefore, compromises in flowsheet design must be made based on the operating parameters and offgas characteristics of each individual facility" @default.
- W90171716 created "2016-06-24" @default.
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- W90171716 date "1987-01-01" @default.
- W90171716 modified "2023-09-26" @default.
- W90171716 title "Optimization of NO/sub x/ and iodine removal in nuclear fuel reprocessing" @default.
- W90171716 hasPublicationYear "1987" @default.
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