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- W90968620 abstract "Positive and negative ions of PAH+ have been analysed in low-pressure premixed flames of various fuels. Mass spectra were taken through a molecular beam sampling system by a linear time-of-flight mass spectrometer and reflectron mass spectrometer. The main formation of PAH+ occurs in the oxidation zone of the flames where their concentrations pass through a maximum. The mass increase of PAH+ is a net result of mass growth, decomposition and oxidation. Therefore, mass growth and diminution of PAH and PAH+ is favored by an (a)increase in concentration of unsaturated small hydrocarbons;(b)increase in concentration of unsaturated small hydrocarbon radicals;(c)increase in the size of PAH or PAH+, respectively;(d)increase in temperature (for growth reactions which have an activation energy);(e)increase in temperature which favors thermal decomposition;(f)increase in concentration of oxidizing radicals such as OH;(g)increase in the concentration of O2;(h)decrease in the size (or mass) and in the degree of pericondensation, increase in the number of side chains." @default.
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- W90968620 date "1994-01-01" @default.
- W90968620 modified "2023-09-25" @default.
- W90968620 title "Growth of Large Ionic Polycyclic Aromatic Hydrocarbons in Sooting Flames" @default.
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- W90968620 doi "https://doi.org/10.1007/978-3-642-85167-4_5" @default.
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