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- W918083782 abstract "Photoionization experiments on free molecules and clusters carried out by the author are reviewed. Vibrationally resolved photoelectron spectroscopy with an instrumental resolution below the lifetime broadening has been performed on the core levels of small C, N, and O containing molecules. Subtle details of the interplay between vibrational and electronic structure have been revealed. Probing the carbon core levels of chiral, somewhat larger molecules with circularly polarized synchrotron radiation shows a circular dichroism in the photoelectron angular distribution, which is present even for non-oriented molecular samples. More details on photoionization processes can be revealed by coincidence experiments. Energy spectra of oxygen resonant Auger electrons taken with high resolution and with kinematical reconstruction of the molecular axis directions show clear signatures for intramolecular electron scattering and electron transfer. Photoelectron spectroscopy of clusters at photon energies larger than the He Iα line has rarely been carried out so far. First experiments have proven the existence of a non-local autoionization process – Interatomic Coulombic Decay – which involves cooperative transitions at two different sites of a weakly bonded system." @default.
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- W918083782 date "2005-01-01" @default.
- W918083782 modified "2023-09-27" @default.
- W918083782 title "Photoionization of Molecules and Clusters at a Third Generation Synchrotron Radiation Source" @default.
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