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- W95370438 abstract "Lower explosion limits in hydrogen-oxygen and deuterium-oxygen mixtures have been measured in the diffusion régime. From the data, rate constants are calculated for the reactions H+O2 →OH+O and D+O 2 →OD+O between 800° and 1 000°K. Activation energies are found to differ by the difference in zero-point energies of OH and OD. Temperature-independent pre-exponential factors differ by a factor of two. Transition states of fixed geometry are not reconcilable with the observed kinetics; nor is the classical collision theory. With a transition state of very loose structure, the observed rate constants can be explained and successfully extrapolated down to 300°K and up to 1 650°K." @default.
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- W95370438 date "1968-10-01" @default.
- W95370438 modified "2023-09-26" @default.
- W95370438 title "Kinetics of the branching step in the hydrogen-oxygen reaction" @default.
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- W95370438 doi "https://doi.org/10.1016/0010-2180(68)90061-8" @default.
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