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- W955606341 abstract "We studied the translational and rotational diffusion of gold nanorods within a rod/sphere composite liquid using fluctuation correlation spectroscopy (FCS). The nanorods of length L ∼ 60 nm and diameter d ∼ 17 nm were used at a fixed concentration of ∼1 pM. The concentration of colloidal Ludox spheres (size ∼ 26 nm) was varied up to a volume fraction of ϕ = 0.3 or approximately 7 spheres/L(3). Our experiments showed significant translational anisotropy as the sphere concentration was increased. The translational diffusion parallel to the rod axis (D(T∥)) followed very close to the bulk viscosity of the solution. However, the diffusion normal to the rod axis (D(T⊥)) experienced a significantly higher frictional force. For volume fraction ϕ > 0.1 a slightly modified caging theory by Pecora and Deutch could explain the rotational diffusion of the rods very well. At low volume fraction the agreement is poor, which we interpreted as modification of the local ordering of the spheres, which can affect the rod rotation." @default.
- W955606341 created "2016-06-24" @default.
- W955606341 creator A5008579876 @default.
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- W955606341 date "2015-08-06" @default.
- W955606341 modified "2023-09-24" @default.
- W955606341 title "Translational Anisotropy and Rotational Diffusion of Gold Nanorods in Colloidal Sphere Solutions" @default.
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- W955606341 doi "https://doi.org/10.1021/acs.langmuir.5b01682" @default.
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