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- W96799374 abstract "Simulations predict maximum C 2 -C 10 yields of 14% for both homogeneous and surfaceinitiated CH 4 pyrolysis at 1038 K. Yields are limited by thermodynamics, kinetic inhibition by H 2 , and carbon formation. Continuous H 2 removal from the system can overcome these constraints and increase maximum predicted yields to 88%. CH 4 pyrolysis experiments at 950 K on 4 wt% Mo/H-ZSM5 achieves near-equilibrium conversions (10-12%) with >90% C 2 -C 10 selectivity by catalyzing both C 2 H 4 formation from CH 4 (on MoO x C y ) and C 2 H 4 aromatization (on H + ), while restricting chain growth to benzene and naphthalene. An H-transport membrane reactor of dense SrZr 0.95 Y 0.05 O 3 thin (10-100 μm) films can be used to overcome these thermodynamic constraints. Self-supporting, thick (1000 μm) disks were prepared via combustion synthesis methods, which form denser membranes than powders formed via co-precipitation. Membrane reactor experiments using thick SrZr 0.95 Y 0.05 O 3 disks had H-transport rates insufficient to affect CH 4 pyrolysis reactions." @default.
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- W96799374 date "1998-01-01" @default.
- W96799374 modified "2023-09-23" @default.
- W96799374 title "Non-oxidative catalytic conversion of methane with continuous hydrogen removal" @default.
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- W96799374 doi "https://doi.org/10.1016/s0167-2991(98)80465-5" @default.
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