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• W972841671 abstract "Abstract Current energy production habits deplete fossil fuels and accumulate atmospheric CO 2 , which contribute to the global climate change. Electrochemical fuel production via CO 2 reduction reaction is an idealistic yet an achievable process that mitigates CO 2 emissions and simultaneously satisfies energy demands. Here, the enhancement of CO 2 reduction activity and stability on size-controlled particulate Ag electrocatalysts derived from a simple, one-step cyclic voltammetry (CV) process by changing scan rates (1–200 mV/s) was demonstrated. Interestingly, larger nanoparticles prepared by slower scan rates (1–5 mV/s) have exhibited the most degree of enhancement for CO 2 reduction to CO product. Compared to untreated Ag foil, nanostructured Ag electrode has shown an anodic shift of approximately 200 mV in the onset potential of CO partial current density ( j CO ), 160 mV reduction of overpotential at j CO  = 10 mA/cm 2 , and increased Faradaic efficiency (F.E.) for CO production especially at lower biased potentials (−0.89 to −1.19 V vs. RHE). Stability tests have demonstrated a drastic improvement in maintaining CO F.E. X-ray photoelectron spectroscopy suggests that the enhancement is associated with stable oxygen species incorporated on the nanoparticle Ag surfaces during the CV fabrication process." @default.
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• W972841671 date "2016-01-01" @default.
• W972841671 modified "2023-10-16" @default.
• W972841671 title "Enhancement in carbon dioxide activity and stability on nanostructured silver electrode and the role of oxygen" @default.
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• W972841671 doi "https://doi.org/10.1016/j.apcatb.2015.06.046" @default.
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