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- W976629897 abstract "Individual and simultaneous hydrodesulfurization (HDS) of dibenzothiophene (DBT) and hydrodenitrogenation (HDN) of carbozole reactions have been studied in the presence of hydrogen (P = 55 bar) at 310 °C in a batch reactor over a series of sulfided NiMo/P/Al-HMS catalysts modified with phosphorus (0.5–2.0 wt%). Both oxidic precursors and sulfide catalysts have been characterized by specific surface area, XRD, Raman, TPD-NH3, HRTEM, XPS and IR spectroscopy of adsorbed pyridine. Regardless of the reaction studied, all P-containing catalysts showed higher activity than that to the P-free one. The catalyst modified with optimized amount of P (1 wt%) the best HDS activity and exhibited a lowest inhibition factor during simultaneous HDS and HDN, which was close to that of a commercial NiMo/Al2O3 sulfide catalyst. This was linked with formation of irregular MoS2 structures having high concentration of brim sites as well as with its largest total acidity." @default.
- W976629897 created "2016-06-24" @default.
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- W976629897 date "2016-01-01" @default.
- W976629897 modified "2023-09-30" @default.
- W976629897 title "Competitive HDS and HDN reactions over NiMoS/HMS-Al catalysts: Diminishing of the inhibition of HDS reaction by support modification with P" @default.
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- W976629897 doi "https://doi.org/10.1016/j.apcatb.2015.07.013" @default.
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