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- W97896320 abstract "Photoassisted solid-catalyzed reduction of nitrogen (pure or in air) to ammonia has been observed using metal oxides as catalysts and liquid or gaseous water as reductant. With alpha-Fe2O3 and Cr2O3, if dissolved ammonia remains in contact with illuminated aqueous suspensions of catalyst, the system achieves a steady concentration of ammonia. When methanol, formaldehyde, glucose or glycerol was dissolved in aqueous suspensions of alpha-Fe2O3 or several other catalysts, or cellulose was suspended in the slurry, up to 30-fold increases in yields of ammonia were obtained upon illumination for 15–34 hrs. When dissolved ammonia remained in contact with illuminated suspensions of alpha-Fe2O3 which contained organic compounds, the rate of production of ammonia increased with time to a maximum and then declined; finally ammonia decayed and disappeared entirely. A maximum rate of production of ammonia per incident photon which has been observed over alpha-Fe2O3 is one fifth of the rate calculated for solar fixation over this catalyst sufficient to supply the nitrogen needs of rice or corn." @default.
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- W97896320 date "1986-01-01" @default.
- W97896320 modified "2023-09-23" @default.
- W97896320 title "PHOTOASSISTED SOLID-CATALYZED REDUCTION OF AIR BY AQUEOUS ORGANIC MATERIALS: A POTENTIALLY PRACTICAL METHOD OF FIXING NITROGEN" @default.
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- W97896320 doi "https://doi.org/10.1016/b978-0-08-033177-5.50353-7" @default.
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