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- W99554102 abstract "Monsanto Research Corporation is charged with processing encapsulated plutonium dioxide heat sources into radioisotopic thermoelectric generators (RTGs) to support deep-space missions. One of the problems associated with the sometimes protracted ground storage of these devices is the ingrowth of carbon dioxide and carbon monoxide in the gas phase due to the cyclical reaction established between the fuel (/sup 238/PuO/sub 2/) and the carbon impact body. This ingrowth proceeds according to the two equations: x(CO) + = x(CO/sub 2/) + < PuO/sub 2-x/ and x(CO/sub 2/) + x < C > = 2x(CO), etc. To reduce this effect, a gas management system was instituted that enabled periodic removal of the generated CO and CO/sub 2/ with replacement by argon. The removal of these components was monitored and permitted an assessment of the degree of substoichiometry as well as its effect on the chemical activity of the CO and CO/sub 2/. This in turn was used to estimate the oxygen activity and to calculate ..delta.. anti G(O/sub 2/) as a function of stoichiometry." @default.
- W99554102 created "2016-06-24" @default.
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- W99554102 date "1982-08-31" @default.
- W99554102 modified "2023-10-06" @default.
- W99554102 title "Behavior of oxygen partial pressure over slightly substoichiometric plutonia at 1410/sup 0/K" @default.
- W99554102 doi "https://doi.org/10.2172/5096006" @default.
- W99554102 hasPublicationYear "1982" @default.
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